Mindscape

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Barbossa is the most exasperated character in any scene he's in, unless he's winning. then he's the smuggest son of a bitch on screen (he literally returns from the dead smugly eating an apple). but majority of the time, he's 'why am I the only adult here'. man rolls his eyes so much I half-expected him to turn straight to the camera.

when Will asks Elizabeth to marry him while they are fighting Davy Jones' crew, stuck in a maelstrom, and trapped in the final battle, the first word out of her mouth is "Barbossa!". she then continues by asking Barbossa to marry them, but for a split second Will's face goes like 'Barbossa? Barbossa?? I didn't even know he was on the map of this convoluted love quadrangle!'

when they're in Singapore and Sao Feng threatens the spy he found and Will, Elizabeth, and Barbossa all look at each other to confirm that none of them have snuck in a spy they forgot to tell the others about, before shrugging and telling Sao Feng to go ahead and kill him.

Barbossa's eyes just getting wide and wider the more weapons Elizabeth pulls out of her clothes. c'mon man, let a woman have her toys!

rewatching really gives you the full picture of how many people are scheming at any given time and how each person's schemes intersect with the others, even if they're nominally on the same side. everyone also gets So Upset when their scheme is foiled, accidentally or intentionally, by someone else's scheme, as though they themselves aren't scheming at that very moment.

Barbossa's iron balls. I'm sorry, this is the funniest dick joke in the trilogy that defines how many dick jokes Disney can stick in a movie before it stops being PG-13. Jack's reaction really says it all.